Oh sorry, I see what you mean. I'd be worried about fitting it, to be honest. I'd much rather just take one drive out and replace it with another drive...
You'd need a 2.5" to 3.5" carriage. They're about US$5 or so.
I'm not that much of a tinkerer! Also 2.5" 1TB drives, are they as reliable as their 3.5" counterparts?
I've had one notebook drive fail (Seagate 80 gb) and four 3.5" drives fail (3 WD, and the infamous Seagate 750 gb firmware problem). I know of no data in terms of reliabilities between the form factors.