From your first post and the diskutil list, it all looks normal. You have
disk0: 28GB This is the SSD part of what was your Fusion Drive (28GB SSD + HDD you removed).
Disk1: 4TB the SATA SSD and it has a single APFS container/partition disk2.
Disk2: Normal result of a macOS install with the disk named as Macintosh 4TB SSD.
What you view in Finder as "Macintosh 4TB SSD" is a combination of two volumes:
disk2s1: Macintosh 4TB SSD (the read only part of macOS), and
disk2s4: Macintosh 4TB SSD - Data (everything else).
This is the bit that many people find "weird".
macOS prevents you (even with admin rights) to create new folders in the root of the system/boot disk. So it is normal that you can't and messing with permissions and ACLs will not change this.
You can create folders under your home directory /Users/whoever, or /Users/Shared, etc.
So everything looks good.
This is what
@chown33 and
@alfogator were trying to explain. I may (or may not) have explained better.

.
Do not be distracted by those showing you how to modify permissions and ACLs on folders, etc.
But, I do note that you do have a bit over 500 GB in use. I assume you know what this is.