This is what I did. It required a reboot, but no reinstall.
I followed e_whizz's instructions (

Thanks!

) and ran into the same problem with the disk not unmounting

. I didn't want to reinstall or boot off of a DVD so I did the following.
1) I downloaded a copy of Carbon Copy Cloner (which everyone should have a copy of) and cloned my boot disk, named "ueberserver" to the secondary disk "Macintosh HD2".
2) When the disk was finished cloning I went into the startup disk control panel and selected "Macintosh HD2" as the boot disk and rebooted the system.
3) Once I was rebooted and using "Macintosh HD2" as my boot disk I ran
diskutil AppleRAID enable mirror disk0s2
And got the following output:
/dev/disk0
#: TYPE NAME SIZE IDENTIFIER
0: GUID_partition_scheme *500.1 GB disk0
1: EFI 209.7 MB disk0s1
2: Apple_HFS ueberserver 499.8 GB disk0s2
/dev/disk1
#: TYPE NAME SIZE IDENTIFIER
0: GUID_partition_scheme *500.1 GB disk1
1: EFI 209.7 MB disk1s1
2: Apple_HFS Macintosh HD2 499.8 GB disk1s2
ueberserver:~ jamie$ diskutil AppleRAID enable mirror disk0s2
Started RAID operation on disk0s2 ueberserver
Resizing disk
Unmounting disk
Adding booter for disk
Creating RAID set
Bringing RAID partition online
Waiting for new RAID to spin up "7B824483-6E4B-4520-BA0F-161DFA51A359"
Finished RAID operation on disk0s2 ueberserver
4) I went back into the Startup Disk control panel and selected the "ueberserver" drive, disk0, as the boot volume and rebooted the system.
5) Once I was rebooted and using the "ueberserver" disk as the boot disk I ran.
diskutil AppleRAID enable mirror disk0s2
The output looked like this:
Started RAID operation on disk0s2 ueberserver
Resizing disk
Unmounting disk
Adding booter for disk
Creating RAID set
Bringing RAID partition online
Waiting for new RAID to spin up "7B824483-6E4B-4520-BA0F-161DFA51A359"
Finished RAID operation on disk0s2 ueberserver
6) Running
diskutil AppleRAID list
Produced this output
AppleRAID sets (1 found)
===============================================================================
Name: ueberserver
Unique ID: 7B824483-6E4B-4520-BA0F-161DFA51A359
Type: Mirror
Status: Degraded
Size: 499.8 GB (499763871744 Bytes)
Rebuild: manual
Device Node: disk2
-------------------------------------------------------------------------------
# Device Node UUID Status
-------------------------------------------------------------------------------
0 disk0s2 9E911EC2-F3D2-4EDA-BDF0-03419FAD1BA5 Online
1 disk1s2 DEFD4471-7E67-48C3-A6B4-06DE32F1B06F 0% (FAILED)
===============================================================================
The second disk was showing as failed because it had data on it. I could have fixed this from the command line but instead went into Disk Utility and told it to rebuild the RAID mirror. Disk Utility warned me that doing so would erase all of the data on disk1s2, which I was OK with, and I clicked OK and off it went.
7) After telling disk utility to rebuild the RAID set
diskutil AppleRAID list
showed the following output:
AppleRAID sets (1 found)
===============================================================================
Name: ueberserver
Unique ID: 7B824483-6E4B-4520-BA0F-161DFA51A359
Type: Mirror
Status: Degraded
Size: 499.8 GB (499763871744 Bytes)
Rebuild: manual
Device Node: disk2
-------------------------------------------------------------------------------
# Device Node UUID Status
-------------------------------------------------------------------------------
0 disk0s2 9E911EC2-F3D2-4EDA-BDF0-03419FAD1BA5 Online
1 disk1s2 DEFD4471-7E67-48C3-A6B4-06DE32F1B06F 8% (Rebuilding)
===============================================================================
Thanks to e_whizz for posting some great instructions and to the nice folks who write Carbon Copy Cloner (throw some bucks their way, this utility can save your butt). I'm stumped as to why some people were able to run this without issue, the only thing I can think of that might have caused this, which I didn't think of until after I had gone through the steps listed above, was to run the initial diskutil command , was to run the initial
diskutil AppleRAID enable mirror disk0s2
with sudo. Perhaps the failure to unmount was a permissions problem, although that seems unlikely.