You're most likely going to need to use Redsn0w to jailbreak and "hactivate" it, so that you can see the Springboard. You will also need to use Redsn0w to install the iPad baseband. The iPad bb will allow for the unlock to happen. Your new baseband is not supported by Ultrasn0w. With the iPad baseband you will lose your GPS functionality and you will only be able to restore/update to custom firmware that is created with pwnagetool (Mac) or Sn0wbreeze (Win). Once you're jailbroken, install Ultrasn0w through Cydia.
You will need a 4.3.3 IPSW for Redsn0w to read. It can be found here:
http://www.felixbruns.de/iPod/firmware/