While I'm not as lucky as Phrasikleia to have both the 5DII and 7D in my possession, I did just switch from a 5DII to a 7D.
Simply put: I grew tired of missing the focus on shots.
So I switched to a 7D. Instantly I'm getting a much much larger percentage of in-focus shots. The AF speed is really not a factor with portraits/landscapes as the actual speed is determined by the lens itself (the tracking speed/accuracy is where the 7D is phenomenal) however, the ability to use any focus point is huge, and they're all accurate.
Interesting and very helpful. I seldom hear of people switching in this direction. But one of the things I'd like to improve, not make worse, is keepers of my GF in low light (restaurant or bar) where I'm using razor thin DOF with the 35L at f1.4-f2. Sounds like it will be tough to beat the performance of the 7D here. That added stop of high ISO image quality doesn't matter if I have to reject the pic because it's OOF.
Just as a matter of principle, I would try to suppress your gear lust and wait out until the 7D is long in the tooth, it is a terrific camera. In the meantime, save up the necessary cash for a 5D Mark III or IV. Even though there may be some improvements in IQ, they will be noticeable only in more challenging situations: if you shoot at low ISO with good glass (which you do have), there will be little improvement. You have proper lenses on a modern camera, and unless you're missing something very specific, I don't haven't seen any particular reason in your post why you have to upgrade to the 5D Mark II.
If you like portraits, the improved AF system of the 7D may actually help you. When I upgraded from a D80 to my D7000, I noticed a marked improvements in AF accuracy: I can nail more shots and set the focus exactly where I want it to be. Two weeks ago, I was shooting a wedding and I was impressed by the number of keeps. Going from a 7D to a 5D Mark II would roughly be the reverse in terms of AF system.
Again, this is a very good point.