What would be the benefit? There is zero reason to upgrade Finder and iTunes to 64-Bit versions, because they wouldn't benefit from it at all. It would only add more development and debugging complexity to applications that just do not require the wider address range for the things that they do.
Video editing, image processing and huge hard disk recording projects can take advantage of a 64-Bit address space. File copying and simple audio playback certainly don't.
If Finder finally became truly multi-threaded, now THAT would bring some directly noticeable benefits and it would immediately reduce the amounts of spinning beach balls that we always have to see.
With 10.6 the finder became a 64 bit app.